the Messenger of Allah (saas) said: "The Greatest Name of Allah is in these two Verses: And your Ilah (God) is One Ilah (God - Allah), La Ilaha Illa Huwa (none has the right to be worshipped but He), the Most Gracious, the Most Merciful.' And at the beginning of Surah Al 'Imran."
Sunan Ibn Majah Book 34, Hadith 29